Development of a macro and microscopic approach to investigate the geochemistry of radioactive waste disposal systems

 

Articles

Osán J, Kéri A, Breitner D, Fábián M, Dähn R, Simon R, Török S
Microscale analysis of metal uptake by argillaceous rocks using positive matrix factorization of microscopic X-ray fluorescence elemental maps
Spectrochimica Acta Part B 91 (2014) 12-23.
DOI: 10.1016/j.sab.2013.11.002

Breitner D, Osán J, Fábián M, Zagyvai P, Szabó C, Dähn R, Marques Fernandes M, Sajó I, Máthé Z, Török S
Characteristics of uranium uptake of Boda Claystone Formation as the candidate host rock of high level radioactive waste repository in Hungary
Environmental Earth Sciences 73 (2015) 209-219
DOI: 10.1007/s12665-014-3413-4

Van Loon LR, Mibus J
A modified version of Archie's law to estimate effective diffusion coefficients of radionuclides in argillaceous rocks and its application in safety analysis studies
Applied Geochemistry 59 (2015) 85-94
DOI: 10.1016/j.apgeochem.2015.04.002

Marques Fernandes M, Vér N, Baeyens B
Predicting the uptake of Cs, Ni, Co, Eu, Th and U on argillaceous rocks using sorption models for illite
Applied Geochemistry 59 (2015) 189-199
DOI: 10.1016/j.apgeochem.2015.05.006

Kéri A, Osán J, Fábián M, Dähn R, Török S
Combined X-ray microanalysis study of the Nd uptake capability of argillaceous rocks
X-Ray Spectrometry 45 (2016) 54-62
DOI: 10.1002/xrs.2656

Gergely F, Osán J, Szabó BK, Török S
Analytical performance of a versatile laboratory microscopic X-ray fluorescence system for metal uptake studies on argillaceous rocks
Spectrochimica Acta Part B 116 (2016) 75-84
DOI: 10.1016/j.sab.2015.12.007

Németh T, Máthé Z, Pekker P, Dódony I, Kovács-Kis V, Sipos P, Cora I, Kovács I
Clay mineralogy of the Boda Claystone Formation (Mecsek Mts., SW Hungary)
Open Geosciences 8 (2016) 259-274
DOI: 10.1515/geo-2016-0024

Proceedings papers

Breitner D, Osán J, Török S, Sajó I, Dähn R, Máthé Z, Szabó C
X-Ray Microspectroscopic Investigations of Ni(II) uptake by Argillaceous Rocks of the Boda Silstone Formation in Hungary
in: Clay characterisation from nanoscopic to microscopic resolution, NEA Clay Club Proceedings 2011.
NEA/RWM/CLAYCLUB(2013)1, OECD NEA, 2013, pp. 58-61.
[Full text]

Máthé Z, Varga A
Mineralogical and petrological characterization of Boda claystone Formation (BCF) and preliminary sketch of its diagenesis
in: Dályay V, Sámson M, Hámos G, eds.
IV. Kõzettani és Geokémiai Vándorgyûlés kiadványa, Molnár Nyomda és Kiadó Kft., Pécs, 2013, ISBN 978-963-8221-52-0
[in Hungarian]

Gergely F, Osán J, Fábián M, Török Sz, Baeyens B, Dähn R, Marques M
High level waste disposal in deep geological waste repository in claystone
in: Bitay E, Szilágyi J, Talpas J, eds.
FMTÜ XIX. Nemzetközi Tudományos Konferencia Kiadványa, Erdélyi Múzeum-Egyesület, Kolozsvár, 2014, ISSN 2067-6808
[in Hungarian]
[Full text]

Abstracts in periodicals

Dähn R, Osán J, Breitner D, Sajó I, Marques M, Baeyens B, Török S
X-ray microspectroscopic investigations of Ni(II) uptake by argillaceous rocks of the Boda Claystone Formation in Hungary
Mineralogical Magazine, 76 (2012) 1613

Marques Fernandes M, Dähn R, Vér N, Baeyens B
Bottom up Approach for the Predictive Modelling of Sorption Isotherms on Argillaceous Rocks
Mineralogical Magazine 77(5) (2013) 1687

University textbooks

Zagyvai P, Kókai Zs, Hózer Z, Breitner D, Fábián M, Török Sz, Börcsök E
Radiactive waste of nuclear fuel cycle
HAS Centre for Energy Research, Budapest, 2013, 146 p.
ISBN:978-963-7351-20-4
[in Hungarian]
[Download PDF]

Annual reports

Osán J, Dähn R, Breitner D, Sajó I, Borchert M, Appel K
Micro-XRF and micro-EXAFS study of the uptake of nickel by argillaceous rocks
HASYLAB Annual Report 2010, paper 20101266
[Full text]

Osán J, Breitner D, Török S, Dähn R, Sajó IE, Simon R
Micro-XRF and micro-XRD study of the uptake of nickel and uranium by argillaceous rocks
ANKA Annual Report 2011
[Full text]

Osán J, Dähn R, Breitner D, Soltermann D, Wieland E, Török S, Borchert M, Appel K
Microspectroscopic study of the uptake of nickel by the host rock of Boda Siltstone Formation, Hungary
HASYLAB Annual Report 2011, paper 20111761
[Full text]

Osán J, Dähn R, Breitner D, Sajó IE, Borchert M, Appel K
Micro-XRF and micro-XRD study of the uptake of nickel and uranium by argillaceous rocks
HASYLAB Annual Report 2011, paper 20111759
[Full text]

Osán J, Breitner D, Fábián M, Gergely F, Dähn R, Marques M, Simon R
Micro-XRF and micro-XRD study of the uptake of radionuclides by argillaceous rocks
ANKA User Reports 2012-2013, pp. 63-64
[Full text]

Osán J, Fábián M, Török S, Gergely F, Kéri A, Dähn R, Simon R
Micro-XRF and micro-XRD study of the uptake of radionuclides by argillaceous rocks
ANKA User Reports 2012-2013, pp. 168-169
[Full text]

Osán J, Marques Fernandes M, Dähn R, Eltayeb E, Szabó Á, Steininger R, Göttlicher J
Micro-EXAFS study of the uptake of radionuclides by argillaceous rocks
ANKA User Reports 2012-2013, pp. 170-171
[Full text]

Conference presentations

Breitner D, Osán J, Török S, Sajó IE, Dähn R, Máthé Z, Szabó C
X-ray microanalytical study of Ni(II) sorption onto argillaceous rock
of Boda Siltstone Formation, Hungary
poster
Multinational Congress on Microscopy (MCM 2011), Urbino, Italy, 04-09 09 2011

Török S, Breitner D, Répánszki R, Osán J, Dähn R, Sajó I
Micro-XRF and micro-EXAFS investigations of radionuclide sorption in Boda Siltstone Formation
talk
3rd International Nuclear Chemistry Congress (3rd-INCC), Palermo, Italy, 18-23 09 2011

Breitner D, Osán J, Török S, Sajó IE, Dähn R, Máthé Z, Szabó C
X-ray microanalytical study of Ni(II) sorption onto argillaceous rock
of Boda Siltstone Formation, Hungary
poster
NEA Clay Club Workshop on Microscopic Observations and Imaging Techniques, Karlsruhe, Germany, 6-8 09 2011

Osán J, Breitner D, Dähn R, Kéri A, Sajó IE, Fábián M, Török S
X-ray microspectroscopic investigation of the uptake of Cs(I), Ni(II), Nd(III) and U(VI) by argillaceous rocks of the Boda Siltstone Formation, Hungary
talk
European Conference on X-ray Spectrometry, Vienna, Austria, 18-22 June 2012

Dähn R, Osán J, Breitner D, Sajó I, Marques M, Baeyens B, Török S
X-ray microspectroscopic investigations of Ni(II) uptake by argillaceous rocks of the Boda Claystone Formation in Hungary
poster
22nd Annual V. M. Goldschmidt Conference, Montreal, Canada, 24-29 June 2012

Breitner D, Osán J, Fábián M, Sajó I, Marques M, Dähn R, Szabó C, Máthé Z, Török S
Retention mechanisms of U(VI) in Boda Claystone Formation as the candidate host rock of high activity and long lived nuclear waste repository in Hungary
poster
34th International Geological Congress, Brisbane, Australia, 5-10 August 2012

Németh T, Dódony I, Máthé Z
Detailed study of clay minerals in Boda Siltstone Formation, possible repository of high level nuclear waste in Hungary
poster
6th Mid-European Clay Conference (MECC’12), Pruhonice, Czech Republic, 4-9 September 2012

Dähn R
The use of X-ray absorption spectroscopy from the bulk- to the nano-scale to study radioactive waste repository materials
talk
School on Synchrotron Radiation Methods and their Applications in Earth Science 2012, Mátrafüred, Hungary, 24-26 September 2012

Marques Fernandes M, Ver N, Baeyens B
Application of the “bottom up” approach for the predictive modelling of sorption isotherms on Hungarian Boda Clay
poster
5th International Meeting on Clays in Natural & Engineered Barriers for Radioactive Waste Confinement, Montpellier, France, 22-25 October 2012

Osán J, Kéri A, Breitner D, Fábián M, Dähn R, Török S
Microscale mineral analysis of clay rock thin sections after sorption experiment using SRXRF
talk
Colloquium Spectroscopicum Internationale XXXVIII (CSI XXXVIII), Tromsø, Norway, 27–30 June 2013

Osán J, Kéri A, Breitner D, Fábián M, Dähn R, Török S
Microscale characterization of radionuclide uptake in Boda Claystone Formation using synchrotron radiation [in Hungarian]
invited talk
Conference of Hungarian Physicists, Debrecen, Hungary, 21-24 August 2013

Marques Fernandes M, Dähn R, Ver N, Baeyens B
Bottom up Approach for the Predictive Modelling of Sorption Isotherms on Argillaceous Rocks
invited talk
23rd Goldschmidt International Conference, Florence, Italy, 25-30 August 2013

Dähn R.
Validation of uptake processes of radionuclides such as Cs on clay minerals by EXAFS
invited talk
Fukushima recovery – understanding, modeling and managing radiocaesium decontamination workshop, Fukushima, Japan, 30 September-3 October 2013

Dähn, R.
Uptake and alteration processes in Opalinus clay: An x-ray absorption and micro-x-ray-diffraction study
invited talk
50th Annual Meeting of the Clay Minerals Society, Urbana, USA, 6-10 October 2013

Gergely F et al.
High level waste disposal in clay formation [in Hungarian]
talk
XX. FMTÜ, Cluj Napoca, Romania, 19-20 March 2014

Osán J, Kéri A, Fábián M, Dähn R, Török S
Microscale analysis of U(VI) uptake by argillaceous rocks using synchrotron radiation X-Ray methods
invited talk
Actinide XAS 2014, Scloss Böttstein, Switzerland, 20-22 May 2014

Kéri A, Osán J, Fábián M, Dähn R, Török S
Application of positive matrix factorization and microscopic X-Ray fluorescence spectroscopy in the examination of argillaceous rocks
poster
Actinide XAS 2014, Scloss Böttstein, Switzerland, 20-22 May 2014

Osán J, Török S, Dähn R, Baeyens B
X-ray spectrometry investigation of radionuclide uptake on argillaceous rocks
invited talk
EXRS 2014, Bologna, Italy, 15-20 June 2014

Osán J, Kéri A, Fábián M, Dähn R, Török S
Microspectrometry investigation of clay-rich rock thin sections after sorption experiment
poster
IGDTP GeoDisposal 2014, Manchester, UK, 24-26 June 2014

Dähn R, Osán J, Pattison P, Wieland E
The challenge of analyzing microdiffraction patterns: From argillaceous rock formations to cement-clay interfaces
talk
Clay Conference 2015, Brussels, Belgium, 23-26 March 2015

Gergely F, Osán J, Kéri A, Dähn R, Fábián M, Török S
Microscale X-ray analysis of metal uptake by argillaceous rocks
poster
Euroclay 2015 - international conference on clay science and technology, Edinburgh, UK, 5-10 July 2015

Dähn R, Osán J, Marques Fernandes M, Baeyens B, Török S
X-ray microspectroscopic investigations of heavy metal uptake by argillaceous rocks
talk
16th International Conference on X-ray Absorption Fine Structure (XAFS16), Karlsruhe, Germany, 23-28 August 2015

Osán J, Kéri A, Fábián M, Gergely F, Dähn R, Grolimund D, Simon R, Török S
Combined X-ray microanalytical study of metal uptake capability of argillaceous rocks
poster
Colloquium Spectroscopicum Internationale XXXIX (CSI 2015), Figueira da Foz, Portugal, 30 August - 3 September 2015

Gergely F, Osán J, Dähn R, Fábián M, Grolimund D, Kéri A, Török S
Microscale X-ray spectrometry investigation of radionuclide uptake on argillaceous rocks
talk
European Symposium on Atomic Spectrometry (ESAS 2016), Eger, Hungary, 31 March - 2 April 2016